洞庭湖及其支流沉积物重金属污染分布特征、风险及影响因子分析
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本文为中国地质调查局项目(编号:No. DD20230478)、湖南省自然科学基金(编号:2024JJ7620)的成果


Distribution characteristics and risk of heavy metal pollution in the sediments of Dongting Lake and its tributaries and the impact factor analysis
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    摘要:

    洞庭湖区为我国重要的“鱼米之乡”,也是主要粮食生产区之一。近年来,伴随着经济的快速发展,洞庭湖及其支流重金属污染时有发生,特别是沿流域工业、生活污水的乱排滥放,导致流域重金属污染日益严重。重金属在自然界很难分解和易通过食物链累积,最终可能危害人体健康。而河流表层沉积物是重金属的“源和汇”,极易续集和二次释放。本文以洞庭湖流域为研究区,系统采集表层沉积物样品,通过地积累指数法、地理探测器、地理加权回归探究其重金属分布特征、污染现状及影响因素驱动分析,以期为相关部门抉择治理提供指导。经研究发现:洞庭湖及其支流沉积物Cd、Cr、Cu、Mn、Ni、Pb、Zn 七种重金属含量分别是洞庭湖水系底泥背景值的5. 06、1. 69、1. 74、2. 02、1. 54、1. 58、1. 67倍。重金属Cd元素为背景值的5倍,个别点位超过土壤筛选值,已对周边环境造成危害。Mn为背景值的2倍,在洞庭湖流域增长较快,需要加强监测;通过Igeo(地积累指数)计算,研究区Cd元素的均值在1~2之间,属于中等污染,研究区沉积物重金属Cr、Cu、Mn、Ni、Pb、Zn元素的Igeo均小于1,均属于轻度污染,洞庭湖及其支流沉积物重金属主要污染物Cd。整体上来看,洞庭湖区各水系沉积物中重金属污染风险较高,整体呈现逐渐积累过程,且基本上处于轻度—偏中度污染水平。通过地理探测器模型发现,降雨、距乡镇距离、气温、据道路距离、土地利用类型、据铁路距离、NDVI、DEM对洞庭湖区沉积物重金属地积累指数(Igeo)具有较强的解释力,表明洞庭湖区沉积物重金属污染受到地理条件等自然因子的影响,同时也与人为活动密切相关;通过地理探测器,筛选出降雨、据公路距离、DEM等对沉积物重金属Itot空间分布解释力强的因子,年平均降雨量和距道路距离是双因子增强的效果外,其他因子交互作用均为非线性增强,表明选取的环境、自然因子共同对湖区表层沉积物重金属空间分布离散发挥一定的驱动作用。

    Abstract:

    To study the distribution characteristics, risks and driving force of heavy metal pollution in the sediments of the Dongting Lake and its tributaries can provide a scientific scheme for the treatment of heavy metal pollution in the surface sediments of the basin, and plays a vital role in ensuring the ecological security of the basin.Methods: This paper evaluates the content of 7 kinds of heavy metal elements in the Dongting Lake Basin, combined with different distribution characteristics. Introduce geographic detector model for spatial differentiation of surface sediments, combined with the Igeo and geographical weighted regression model, quantitative explore various influence factors on the geographical space of the lake surface sediments of heavy metal pollution distribution driver, and the Arcgis of the main influence factor correlation coefficient of spatial visual expression.Results: ① The content of heavy metals in Cd, Cr, Cu, Mn, Ni, Ni, Zn and Zn are 5.06, 1.69, 1.74, 2.02, 1.54, 1.58 and 1.67 times of the background values of sediment in the Dongting Lake water system, respectively. The heavy metal Cd element is 5 times of the background value, and some points exceed the soil screening value, which has caused harm to the surrounding environment. Mn is twice the background value, which grows rapidly in the Dongting Lake basin and requires enhanced monitoring. ② Calculated by Igeo (Earth accumulation index), the mean value of Cd elements in the study area is between 1 and 2, which belongs to moderate pollution. Igeo of heavy metals Cr, Cu, Mn, Ni, Pb and Zn in the study area are less than 1, all belonging to mild pollution, the main heavy pollutant Cd of sediments in the Dongting Lake and its tributaries. On the whole, the risk of heavy metal pollution in the sediments in the Dongting Lake area is high, showing the overall gradual accumulation process, and basically at the mild- moderate pollution level. ③ through the geographic detector model, rainfall, distance from the villages and towns, air temperature, according to the road distance, land use type, according to the railway distance (0.16), NDVI, DEM on the Dongting Lake sediment heavy metal accumulation index (Igeo) has strong interpretation, shows that the Dongting Lake sediment heavy metal pollution by geographical conditions such as natural factors, but also closely related to human activities.Conclusions: ① On the whole, the average value of all elements in the sediments in the Dongting Lake area is 2, which belongs to the medium pollution degree. ② The serious pollution areas are mainly concentrated in the Zijiang River basin and the Xiangjiang River into the Dongting Lake basin and the center of the Dongting Lake, and the sediment sediment in the Yuanjiang River basin shows moderate pollution. ③ through the geographical detector, select rainfall, according to the highway distance, DEM of sediment heavy metal Itot spatial distribution of strong factors, annual average rainfall and distance from the road is the effect of double factor enhancement, other factors interaction are nonlinear enhancement, shows that the selection of environment and natural factors on the lake surface sediment of heavy metal spatial distribution discrete play a driving role.

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引用本文

陈方伟,李聪,郭军,张程安,毛雄,汤恒佳,廖琦,陈创.2025.洞庭湖及其支流沉积物重金属污染分布特征、风险及影响因子分析[J].地质论评,71(1):2025010015,[DOI].
CHEN Fangwei, LI Cong, GUO Jun, ZHANG Cheng’an, MAO Xiong, TANG Hengjia, LIAO Qi, CHEN Chuang.2025. Distribution characteristics and risk of heavy metal pollution in the sediments of Dongting Lake and its tributaries and the impact factor analysis[J]. Geological Review,71(1):2025010015.

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  • 收稿日期:2024-09-23
  • 最后修改日期:2024-12-08
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  • 在线发布日期: 2025-01-19
  • 出版日期: 2025-01-15