富铀花岗岩定年的几种方法对比——以赣中紫云山花岗岩为例
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东华理工大学

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国家自然科学基金项目(41972071),江西省自然科学基金项目(编号:20242BAB26048、 20252BAC240267、 20242BAB20132)


Comparison of Geochronological Methods for Uranium-rich Granites: A Case Study from the Ziyunshan Uranium-rich Granite in Central Jiangxi Province*
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East China University of Technology

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    摘要:

    富铀花岗岩中锆石常因铀含量高而发生强烈蜕晶质化,导致U-Pb定年结果不可信,难以准确获得岩体锆石的U-Pb年龄。为解决高铀花岗岩精确定年难题,本研究以赣中紫云山富铀岩体为研究对象,开展系统的岩相学与岩石地球化学分析,确认其为典型富铀过铝质花岗岩。通过α径迹蚀刻技术定位载铀矿物,结合扫描电镜与电子探针分析,识别出锆石、独居石、磷钇矿、晶质铀矿等原生岩浆矿物,以及铀石、铀钍石等热液次生矿物。针对主要载铀矿物开展定年研究表明:锆石因强烈蜕晶质化,LA-ICP-MS U-Pb年龄分散且偏小(142.8±1.0 Ma),反映其同位素体系未保持封闭;独居石U-Pb加权平均年龄为150.5±0.8 Ma,结果集中可靠;晶质铀矿电子探针U-Th-Pb化学年龄为151.4±1.7 Ma,与前人获得的成岩年龄一致。研究认为,在富铀花岗岩定年工作中,独居石因抗辐照能力强、体系封闭性好,可作为锆石的有效替代定年矿物;晶质铀矿电子探针化学定年也具有较高可行性与准确性,为同类岩体年代学研究提供了重要方法参考。

    Abstract:

    Zircon in uranium-rich granites frequently undergoes intense metamicization owing to elevated uranium content, resulting in unreliable U-Pb dating outcomes and complicating the accurate determination the U-Pb age of zircon from such granite. To tackle the challenges associated with precise dating of high-uranium granites, this study investigates the Ziyunshan pluton in central Jiangxi. Comprehensive petrographic and petrochemical analyses were performed, confirming its classification as a typical uranium-rich peraluminous granite. Using α-track etching technology, uranium-bearing minerals were identified and characterized through scanning electron microscopy and electron probe analysis. These analyses revealed primary magmatic minerals, including zircon, monazite, xenotime, and uraninite, alongside hydrothermal secondary minerals such as coffinite and thorite. Geochronological investigations of the principal uranium-bearing minerals indicated that zircon, affected by intense metamicization, produced scattered and anomalously young LA-ICP-MS U-Pb ages (142.8 ± 1.0 Ma), suggesting an open isotopic system. In contrast, monazite yielded a weighted average age of 150.5 ± 0.8 Ma, which is both consistent and reliable. Additionally, the electron probe U-Th-Pb chemical age of uraninite was determined as 151.4 ± 1.7 Ma, aligning with previously established rock formation ages. This study demonstrates that monazite, owing to its strong radiation resistance and robust isotopic system, can serve as an effective alternative to zircon for dating uranium-rich granites. Furthermore, electron probe chemical dating of uraninite proves to be a feasible and accurate method, offering valuable insights for geochronological studies of similar granite.

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  • 收稿日期:2025-10-25
  • 最后修改日期:2025-11-20
  • 录用日期:2025-11-21
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