两花岗岩体接触带铀系核素迁移的初步模拟
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A Simplified Modeling for Radionuclide Migration in a Granitic Contact Zone
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    摘要:

    随着世界各国大力发展核电,放射性废料的安全处置已成为当今研究热点和前沿学科。高放废物深地质处置的安全性主要取决于处置库内放射性核素向生物圈的迁移程度。在侵入岩中,放射性核素主要是通过地下水沿岩石孔隙从处置库向生物圈迁移的。为了理解放射性核素在花岗岩体接触带的迁移行为,本文根据两花岗岩体接触带中样品的铀系核素放射性活度比值(^234U/^238U,^230Th/^234U,^226Ra/^230Th,^230Th/^238U),利用 α-反冲(弹射)作用引起的放射性不平衡理论,计算了铀系核素子体^234U,^230Th,^226Ra在后期地下水的作用下在花岗岩体接触带及其裂隙内的迁出率、迁入率、并进行了质量平衡的计算。结果表明,经α-反冲作用进入流体的核素的迁出率要远大于因核素自然衰变的消亡率;裂隙充填物及裂隙能阻滞大量核素的迁移,其沉淀核素来自接触带花岗岩;花岗岩能强烈阻滞核素的迁移,可作为阻止放射性核素从核废料地下处置库向外迁移的有利天然屏障。

    Abstract:

    With the great development of nuclear power, radwaste safety disposal has become an advanced research hotspot worldwidely. Safety performance of a deep geology disposal vault is mainly dependent on the degree of radionuclide migration from the vault to biosphere. As pluton rocks, the radionuclides in disposal were transported from deep geological media to biosphere mainly by groundwater through rock fracture or contact plane. In order to interpret and predict th e radionuclide migration behaviour in granitic contact zone, the removal ratios and input ratios of 226Ra, 234U and 230Th in granite bodies and in their fracture are calculated according to a model based on a-recoil theory and the measure radionuclide activity ratios of the samples from the Xiangcaoping and Douzhashan granitic bodes. The results are in conformity with the previous conclusions derived from geochemistry study. The results show that the removal ratios of radionuclides caused by a-recoil damage are greater than that by their natural decay, and the fracture coating fillings could retard a considerable amount of radionuclides which came from the granite bodies of contacted zone. Granitic bodies have the great power to retard the migration of radwastes so that they could be served as an effective natural barrier to block the radwaste transport from the deep geological vault to biosphere.

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罗兴章 闵茂中.2001.两花岗岩体接触带铀系核素迁移的初步模拟[J].地质论评,47(6):658-664,[DOI].
LUO Xingzhang, MIN Maozhong Department of Earth Sciences, State Key Laboratory of Mineral Deposit Research, Nanjing University, Nanjing,.2001. A Simplified Modeling for Radionuclide Migration in a Granitic Contact Zone[J]. Geological Review,47(6):658-664.

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